In a very general sense, the TT animated figures look nicer as toys, but the Hasbro ones seem more show accurate.
EG, Hasb Jazz has a lightly matte looking white plastic, while TT has a nicer, cleaner white.
Some of them (like Blurr and Optimus) have got the shiny red paint like in the CHUG line.
If I hadn't seen the TV show, I'd want all the TT versions, as they do look nicer. But since I have, I stuck with the Hasbro as they looked much closer to the show. IMO
Comparison of
Arcees
Ratchet Comparison
Rodimus x three
And a Bumblebee
Hmm, that rhymes a little bit